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Watson–Crick Base-Pairing Properties of Nucleic Acid Analogues with Stereocontrolled α and β Torsion Angles (α,β-D-CNAs)
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Watson–Crick Base-Pairing Properties of Nucleic Acid Analogues with Stereocontrolled α and β Torsion Angles (α,β-D-CNAs)

Christelle Dupouy, Nathalie Tarrat, Marie-Pierre Durrieu, Frédéric Rodriguez, Jean-Marc Escudier et Alain Vigroux
Angewandte Chemie International Edition, Vol.45(22), pp.3623-3627
26/05/2006
PMID: 16639765

Résumé

Chemical Physics Chemical Sciences Life Sciences Physics
Constrained nucleic acids (α,β‐D‐CNAs) have an ethylene bridge that locks the α and β backbone torsion angles of DNA in the canonical (gauche(−),trans) conformation, as in B‐form DNA (see picture), or in the noncanonical (gauche(+),trans) conformation. Canonical α,β‐D‐CNAs enhance the duplex‐forming ability of oligonucleotides with complementary DNA, while noncanonical α,β‐D‐CNAs stabilize distorted B‐DNA structures.

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