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Transition-Metal-Free -Arylation of Enolizable Aryl Ketones and Mechanistic Evidence for a Radical Process
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Transition-Metal-Free -Arylation of Enolizable Aryl Ketones and Mechanistic Evidence for a Radical Process

Martin Pichette Drapeau, Indira Fabre, Laurence Grimaud, Ilaria Ciofini, Thierry Ollevier et Marc Taillefer
Angewandte Chemie International Edition, Vol.54(36), pp.10587-10591
01/09/2015
PMID: 26136406

Résumé

Chemistry Chemistry, Multidisciplinary Physical Sciences Science & Technology
The -arylation of enolizable aryl ketones can be carried out with aryl halides under transition-metal-free conditions using KOtBu in DMF. The -aryl ketones thus obtained can be used for step- and cost-economic syntheses of fused heterocycles and Tamoxifen. Mechanistic studies demonstrate the synergetic role of base and solvent for the initiation of the radical process.

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