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Towards the Total Synthesis of Thuggacin A: Synthesis of the C13-C25 Fragment Bearing All-syn Stereocenters
Journal article   Peer reviewed

Towards the Total Synthesis of Thuggacin A: Synthesis of the C13-C25 Fragment Bearing All-syn Stereocenters

Araceli Zarate-Ruiz, Renata Marcia de Figueiredo, Gilles Niel and Jean-Marc Campagne
SYNLETT, Vol.23(2), pp.219-223
02/01/2012

Abstract

macrolide thuggacin antituberculosis aldolization allenylstannane
The diastereoselective synthesis of the key C13-C25 fragment of thuggacin A is described. Two Evans aldolization steps and a diastereoselective addition of an allenylstannane control the required all-syn configuration of the five contiguous stereocenters.
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