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Synthesis, duplex-forming properties, and enzymatic resistance of oligonucleotides containing N -acylsulfonamide linkages
Article de revue   Open Access   Avec comité de lecture

Synthesis, duplex-forming properties, and enzymatic resistance of oligonucleotides containing N -acylsulfonamide linkages

Romain Amador, Carine Baraguey, Guillaume Clavé et Michael Smietana
Organic & Biomolecular Chemistry, Vol.23(42), pp.9576-9581
2025

Résumé

We report the synthesis of (2-(N-acetylsulfamoyl)ethyl)carbamate (NAC)-linked thymidine dinucleotide via the sulfo-click reaction and its incorporation into DNA oligonucleotides. Thermal denaturation studies indicate modest destabilization at duplex ends (∼1 °C) and stronger effects in the middle (∼7 °C), while the NAC linkage provides complete resistance to nucleases.

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