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Stability Is Not Everything: The Case of the Cyclisation of a Thrombin‐Binding Aptamer
Article de revue   Open Access   Avec comité de lecture

Stability Is Not Everything: The Case of the Cyclisation of a Thrombin‐Binding Aptamer

Claudia Riccardi, Albert Meyer, Jean-Jacques Vasseur, Irene Russo krauss, Luigi Paduano, Rosario Oliva, Luigi Petraccone, François Morvan et Daniela Montesarchio
ChemBioChem
14/05/2019

Résumé

click chemistry cyclization molecular recognition aptamers G-quadruplexes
With the aim of developing a new approach to obtain improved aptamers, a cyclic thrombin-binding aptamer (TBA) analogue (cycTBA) has been prepared by exploiting a copper(I)-assisted azide-alkyne cycloaddition. The markedly increased serum resistance and exceptional thermal stability of the G-quadruplex versus TBA were associated with halved thrombin inhibition, which suggested that some flexibility in the TBA structure was necessary for protein recognition.

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