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Silica hybrid material containing Pd–NHC complex as heterogeneous catalyst for Mizoroki–Heck reactions
Journal article   Peer reviewed

Silica hybrid material containing Pd–NHC complex as heterogeneous catalyst for Mizoroki–Heck reactions

Vivek Polshettiwar, Peter Hesemann and Joël J.E. Moreau
Tetrahedron Letters, Vol.48(31), pp.5363-5366
09/06/2007

Abstract

Silica hybrid materials NHC-catalyst Heck-reaction
A silica hybrid material containing palladium-N-heterocyclic carbene complexes was prepared by the sol–gel transformation of a molecular triethoxysilylated Pd–NHC complex. The material showed high activity as heterogeneous catalyst in Mizoroki–Heck reaction of aryl bromides and -iodides with styrene and methyl acrylate and could be re-used in at least five reaction cycles with unchanged catalytic properties.
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